Document Type

Thesis

Date of Award

8-31-1986

Degree Name

Master of Science in Environmental Engineering - (M.S.)

Department

Civil and Environmental Engineering

First Advisor

Paul N. Cheremisinoff

Second Advisor

Su Ling Cheng

Third Advisor

John W. Liskowitz

Abstract

As part of a program to develop new and more cost-effective dewatering approaches for industrial hazardous wastes, sludges and synthetic "model" materials were analyzed by thermal methods in an attempt to comprehend their water-binding qualities and differentiate free and bound water. These thermal methods included Differential Thermal Analysis (DTA), Thermogravimetric Analysis (TG), and Differential Scanning Calorimetry (DSC). Industrial sludges and laboratory models were compared using both standard heating techniques and subambient cooling (to -60°C). This latter technique provides direct indication of the amount of free water. This information can be very useful in evaluating and improving dewatering techniques for industrial hazardous sludges since waters of different binding strengths are removed with varying degrees of ease.

Based on the limited number of samples investigated, it appears that at least with certain sludges, the differentiation of free and bound water can be made by these techniques. The sludges examined have a ratio of bound water to total water, (i.e., the fraction of total water that is considered bound) ranging from 10 to 100%, averaging 50%. These results suggest that investigation of bound versus free water in any industrial sludge could be a worthwhile part of any sludge dewatering program.

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