Document Type

Thesis

Date of Award

6-30-1959

Degree Name

Master of Science in Chemical Engineering - (M.S.)

Department

Chemical Engineering

First Advisor

Joseph Joffe

Second Advisor

C. L. Mantell

Third Advisor

George C. Keeffe

Abstract

Enthalpies and partial molal enthalpies have been calculated by a combination of analytical and graphical procedures for the methane carbon dioxide binary system at 160°F, and at pressures from 200 to 9000 psia.

Mixtures containing .0852, .19912, .3583 and .6685 weight fraction of methane in carbon dioxide, as well as the pure components were used. The method for calculation of the enthalpies was outlined by Van Ness (1) and involves the application of residuals to the Redlich-Kwong equation of state (2).

The results of this paper illustrate the value of the method as an accurate and reasonably convenient tool. Excellent agreement is found for methane enthalpies with values reported by Sage and Lacey (3).

A comparison of partial molal enthalpies for methane with those of Sage and Lacey for the methane ethane system (3) indicates fairly similar values. This is thought to be due to the proximity of the critical temperatures of ethane and carbon dioxide.

Share

COinS
 
 

To view the content in your browser, please download Adobe Reader or, alternately,
you may Download the file to your hard drive.

NOTE: The latest versions of Adobe Reader do not support viewing PDF files within Firefox on Mac OS and if you are using a modern (Intel) Mac, there is no official plugin for viewing PDF files within the browser window.