Electrocatalytic redox neutral [3 + 2] annulation ofN-cyclopropylanilines and alkenes
Document Type
Article
Publication Date
1-21-2021
Abstract
Although synthetic organic electrochemistry (EC) has advanced significantly, net redox neutral electrosynthesis is quite rare. Two approaches have been employed to achieve this type of electrosynthesis. One relies on turnover of the product by the reactant in a chain mechanism. The other involves both oxidation on the anode and reduction on the cathode in which the radical cation or the radical anion of the product has to migrate between two electrodes. Herein, a home-built electrochemistry/mass spectrometry (EC/MS) platform was used to generate anN-cyclopropylaniline radical cation electrochemically and to monitor its reactivity toward alkenes by mass spectrometry (MS), which led to the discovery of a new redox neutral reaction of intermolecular [3 + 2] annulation ofN-cyclopropylanilines and alkenes to provide an aniline-substituted 5-membered carbocycleviadirect electrolysis (yield up to 81%). A chain mechanism, involving the regeneration of the substrate radical cation and the formation of the neutral product, is shown to be responsible for promoting such a redox neutral annulation reaction, as supported by experimental evidence of EC/MS.
Identifier
85100275325 (Scopus)
Publication Title
Chemical Science
External Full Text Location
https://doi.org/10.1039/d0sc05665k
e-ISSN
20416539
ISSN
20416520
First Page
969
Last Page
975
Issue
3
Volume
12
Grant
1915878
Fund Ref
National Science Foundation
Recommended Citation
Wang, Qi; Wang, Qile; Zhang, Yuexiang; Mohamed, Yasmine M.; Pacheco, Carlos; Zheng, Nan; Zare, Richard N.; and Chen, Hao, "Electrocatalytic redox neutral [3 + 2] annulation ofN-cyclopropylanilines and alkenes" (2021). Faculty Publications. 4376.
https://digitalcommons.njit.edu/fac_pubs/4376