Enhanced Recovery of Aviation Biofuel Precursor Isoprenol Using Nanocarbon-Immobilized Membrane-Based Membrane Distillation
Document Type
Article
Publication Date
2-16-2023
Abstract
This paper demonstrates enhanced removal and recovery of isoprenol by employing nanocarbon-immobilized membranes (NCIM) for air-sparged sweep gas membrane distillation (AS-SGMD). The isoprenol flux, separation factor, and mass transfer coefficient obtained for NCIM were significantly higher compared to plain PTFE membranes under various experimental conditions. Among the two types of nanocarbon-immobilized membranes, namely, graphene oxide-immobilized membrane (GOIM) and carbon nanotube-immobilized membrane (CNIM), GOIM exhibited better performance in terms of isoprenol flux and separation factor. Compared to a plain PTFE membrane, GOIM showed a 71% increase in the isoprenol flux and a 52% increase in the separation factor, achieving a maximum separation factor of 3.6 and flux of 0.68 kg/m2 h at a temperature of 80 °C. Enhanced performance of NCIM is attributed to the alteration of the partitioning effect through preferential sorption of the organic moiety, followed by fast desorption from nanocarbon surfaces. The demonstrated enhancements to both membrane flux and isoprenol concentration factor create the potential for significant capital and operational cost savings if such membranes are deployed at a commercial scale.
Identifier
85147229299 (Scopus)
Publication Title
Energy and Fuels
External Full Text Location
https://doi.org/10.1021/acs.energyfuels.2c03637
e-ISSN
15205029
ISSN
08870624
First Page
2875
Last Page
2885
Issue
4
Volume
37
Grant
CBET-1603314
Fund Ref
National Science Foundation
Recommended Citation
Bhoumick, Mitun Chandra; Li, Cheng; Roy, Sagar; Sundstrom, Eric; Harvey, Benjamin G.; and Mitra, Somenath, "Enhanced Recovery of Aviation Biofuel Precursor Isoprenol Using Nanocarbon-Immobilized Membrane-Based Membrane Distillation" (2023). Faculty Publications. 1913.
https://digitalcommons.njit.edu/fac_pubs/1913