Effects of polymer wrapping and covalent functionalization on the stability of MWCNT in aqueous dispersions

Document Type

Article

Publication Date

3-15-2011

Abstract

The colloidal behavior of aqueous dispersions of functionalized multiwall carbon nanotubes (F-CNTS) formed via carboxylation and polymer wrapping with polyvinyl pyrrolidone (PVP) is presented. The presence of polymer on the nanotube surface provided steric stabilization, and the aggregation behavior of the colloidal system was quite different from its covalently functionalized analog. Based on hydrophobicity index, particle size distribution, zeta potential as well as the aggregation kinetics studied using time-resolved dynamic light scattering, the PVP wrapped CNT was somewhat less prone to agglomeration. However, its long-term stability was lower, and this was attributed to the partial unwrapping of the polyvinyl pyrrolidone layer on the CNT surface. © 2010 Elsevier Inc.

Identifier

79551473550 (Scopus)

Publication Title

Journal of Colloid and Interface Science

External Full Text Location

https://doi.org/10.1016/j.jcis.2010.12.052

ISSN

00219797

PubMed ID

21236442

First Page

383

Last Page

388

Issue

2

Volume

355

Grant

RC2ES018810

Fund Ref

National Institute of Environmental Health Sciences

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