Strain-Control of Cycloidal Spin Order in a Metallic Van der Waals Magnet

Document Type

Article

Publication Date

9-27-2023

Abstract

The manipulation of magnetism through strain control is a captivating area of research with potential applications for low-power devices that do not require dissipative currents. Recent investigations of insulating multiferroics have unveiled tunable relationships among polar lattice distortions, Dzyaloshinskii–Moriya interactions (DMI), and cycloidal spin orders that break inversion symmetry. These findings have raised the possibility of utilizing strain or strain gradient to manipulate intricate magnetic states by changing polarization. However, the effectiveness of manipulating cycloidal spin orders in “metallic” materials with screened magnetism-relevant electric polarization remains uncertain. In this study, the reversible strain control of cycloidal spin textures in a metallic van der Waals magnet, Cr1/3TaS2, through the modulation of polarization and DMI induced by strain is demonstrated. With thermally-induced biaxial strains and isothermally-applied uniaxial strains, systematic manipulation of the sign and wavelength of the cycloidal spin textures is realized, respectively. Additionally, unprecedented reflectivity reduction under strain and domain modification at a record-low current density are also discovered. These findings establish a connection between polarization and cycloidal spins in metallic materials and present a new avenue for utilizing the remarkable tunability of cycloidal magnetic textures and optical functionality in van der Waals metals with strain.

Identifier

85172713201 (Scopus)

Publication Title

Advanced Materials

External Full Text Location

https://doi.org/10.1002/adma.202303750

e-ISSN

15214095

ISSN

09359648

PubMed ID

37358066

Issue

39

Volume

35

Grant

DE‐SC0021188

Fund Ref

U.S. Department of Energy

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